The Sperm Whale (Physeter Macrocephalus) (Cachalot) is the animal with the largest skull in the world (both in general and aquatically).
The African Bush Elephant (Loxodonta Africana) is the largest-skulled terrestrial animal in the world.
The extinct aquatic animal with the largest skull would probably be either a Mosasaurus Hoffmannii or a Carcharodon Megaladon.
The Titanoceratops Ouranos is the extinct terrestrial animal with the largest skull.
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